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31.
32.
Francisco Zaera 《Topics in Catalysis》2005,34(1-4):129-141
Catalysis is central to most industrial processes for chemical manufacturing. As catalytic processes have become more complex and more demanding, selectivity has become the central issue in their design. Selectivity is defined by the relative rates of competing reaction pathways available to crucial intermediates, and can be controlled by subtle changes in the nature of the catalyst, the reactants, and/or the reaction conditions. In order to be able to do this in a systematic manner, a good understanding of the catalytic reaction mechanisms is needed. Here a connection is drawn between the key elementary steps comprising hydrocarbon conversion reactions on surfaces and those known to occur on discrete organometallic complexes. This way, the hydrogenation, dehydrogenation, hydrogenolysis, chain growth, and isomerization reactions typical in heterogeneous catalysis are redefined in terms of hydride elimination, oxidative addition, reductive elimination, migratory insertion, and 1, 2-shift elementary steps, among others. It is suggested that the knowledge already available from organometallic chemistry can be used to further advance the understanding of the surface science involved in heterogeneous catalysis. Thanks to the commonality of the chemistry involved, a better synergy could also be established between homogeneous and heterogeneous catalytic development. These ideas are discussed in this article in a critical and personal way.*Invited contribution to the special volume entitled The Interface between Heterogeneous and Homogeneous Catalysis, stemming from contributions at the recent International Symposium on Relations between Heterogeneous and Homogeneous Catalysis, and dedicated to the memory of Robert L. Burwell. 相似文献
33.
由于恐怖分子利用邮政系统投寄携带炭疽病毒的邮件,传播病毒,已引起美国政府在邮政系统,选择地利用电子辐射杀死病毒。然而,这种病毒袭击并没有得到有效控制,却使信封内的邮件由于高温辐射,受到损坏。有报道说,由于电子辐射使纸张、珠宝、信用卡、软盘和光盘及其它电子材料受到损害。某些研究已在法庭科学中得到验证。本文介绍辐射过程在渗透和非渗透性客体上,对化学试剂、生物酶记录指纹信息的影响。 相似文献
34.
Robert G. Laughlin 《Journal of the American Oil Chemists' Society》1990,67(11):705-710
Recent phase studies of several surfactant-water systems, using new or refined methods, have revealed significant errors in
earlier phase diagrams. These diagrams had been determined largely using methods based on the isoplethal phase studies principle.
This principle has inherent limitations which do not exist in isothermal methods.
Isothermal nuclear magnetic resonance and refined calorimetric methods have been extensively used in recent surfactant phase
studies. Methods based on the new lyotrope gradient (swelling) principle show great promise as a means of improving the efficiency
and quality of surfactant phase studies. 相似文献
35.
B. Naderi M. Zandieh M. Yazdani 《International Transactions in Operational Research》2014,21(6):1031-1044
This paper deals with the presentation of polynomial time (approximation) algorithms for a variant of open‐shop scheduling, where the processing times are only machine‐dependent. This variant of scheduling is called proportionate scheduling and its applications are used in many real‐world environments. This paper develops three polynomial time algorithms for the problem. First, we present a polynomial time algorithm that solves the problem optimally if , where n and m denote the numbers of jobs and machines, respectively. If, on the other hand, , we develop a polynomial time approximation algorithm with a worst‐case performance ratio of that improves the bound existing for general open‐shops. Next, in the case of , we take into account the problem under consideration as a master problem and convert it into a simpler secondary approximation problem. Furthermore, we formulate both the master and secondary problems, and compare their complexity sizes. We finally present another polynomial time algorithm that provides optimal solution for a special case of the problem where . 相似文献
36.
该文对高校科研管理工作进行了详细分析,结合高职院科研工作的特点,设计并开发了基于C/S和B/S混合模式的科研管理信息系统,该系统从某高职院科研管理工作的业务流程和教职工的实际需要出发,设计了相应的功能模块和操作流程,应用了正则表达式技术直接从“知网”提取教职工论文发表信息,节省了数据录入时间. 该系统投入运行近两年,使用结果表明,该科研管理系统使科研管理工作更加规范,工作效率大大提高. 相似文献
37.
Simon Piché 《Chemical engineering science》2005,60(22):6452-6461
The oxidative absorption of hydrogen sulfide (H2S) into a solution of ferric chelate of trans-1,2- diaminocyclohexanetetraacetate (CDTA) was studied in a counter-current laboratory column randomly packed with 15 mm plastic Ralu rings. The present investigation takes concern about the Kraft pulping situation where dilute H2S concentrations are omnipresent in large-volume gas effluents. A fractional two-level factorial approach was instigated to determine the significance of six operating variables, namely the solution's alkalinity (pH; 8.5-10.5), the liquid mass flow rate (L;1.73-), the solution's ionic strength (IC;0.01-), the gas mass flow rate (G;0.19-), the inlet H2S concentration (CH2S,0;70-430 ppm) and the initial ferric CDTA concentration (CFe,0;100 -). Initially, a Plackett-Burman design matrix of seven duplicated experiments revealed that pH is the leading factor controlling the H2S conversion rate while the ionic strength and ferric CDTA concentration effects remained negligible within the factorial domain. Surface response analysis based on 11 duplicated factorial experiments plus 10 central composite trials revealed that the H2S conversion significantly increases with liquid flow rate but decreases with growing H2S load up. Further examination about the influence of ferric CDTA on H2S absorption rate was set up over a broader concentration range (CFe,0;0- at pH of 9.5 and 10.5. It showed good potential at as H2S conversion increased by a significant 25% for both pH values in comparison to pure alkaline solutions containing no ferric CDTA. 相似文献
38.
信息与计算科学专业实践教学体系创新研究探析 总被引:1,自引:0,他引:1
结合专业建设对信息与计算科学专业实践教学的现状及存在的主要问题进行了分析,同时就信息与计算科学专业实践教学体系的主要内容、总体设计和组织管理方面进行了探讨,提出了按模块分层次构建实践教学内容体系的设想,对信息与计算科学专业实践教学有一定的指导意义。 相似文献
39.
许华民 《杭州电子科技大学学报》2009,29(6)
面向作业调度在当今实际生产企业作业车间调度中得到普遍的应用,其基本思想是将作业一个个地安排到工作机器上。该文介绍了一种印染行业的作业车间调度模型及其处理过程,并给出了基于时间槽的求解算法。该算法通过将指定工序的可行调度起始和结束时间以逆排方式安排到有限能力的工作机器上以达到最大接近交货期的目的,通过对每一机器有效时间槽的操作来减少在每一机器上可行时间槽的搜索时间,从而提高了计算效率。 相似文献
40.
快速发展中的工科背景高等院校在统计教育上存在有待改进的地方。以浙江科技学院为例,为培养具有深厚统计学背景的应用型复合人才,在统计教育上作了一些探索:定位于浙江中小企业对统计知识的实际需求;选择注重实际应用的国外经典教材;在教学中注重学生的参与;在实践中培养学生运用统计学知识和统计工具如统计软件的能力。 相似文献